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We propose and demonstrate a general method to calibrate the frequency-dependent response of selfcompensating noble-gas–alkali-metal comagnetometers to arbitrary spin perturbations. This includes magnetic and nonmagnetic perturbations such as rotations and exotic spin interactions. The method is based on a fit of the magnetic field response to an analytical model. The frequency-dependent response of the comagnetometer to arbitrary spin perturbations can be inferred using the fit parameters. We demonstrate the effectiveness of this method by comparing the inferred rotation response to an experimental measurement of the rotation response. Our results show that experiments relying on zero-frequency calibration of the comagnetometer response can over- or underestimate the comagnetometer sensitivity by orders of magnitude over a wide frequency range. Moreover, this discrepancy accumulates over time as operational parameters tend to drift during comagnetometer operation. The demonstrated calibration protocol enables accurate prediction and control of comagnetometer sensitivity to, for example, ultralight bosonic dark-matter fields coupling to electron or nuclear spins, as well as accurate monitoring and control of the relevant system parameters. 

Abstract Ultralight bosons such as axion-like particles are viable candidates for dark matter. They can form stable, macroscopic field configurations in the form of topological defects that could concentrate the dark matter density into many distinct, compact spatial regions that are small compared with the Galaxy but much larger than the Earth. Here we report the results of the search for transient signals from the domain walls of axion-like particles by using the global network of optical magnetometers for exotic (GNOME) physics searches. We search the data, consisting of correlated measurements from optical atomic magnetometers located in laboratories all over the world, for patterns of signals propagating through the network consistent with domain walls. The analysis of these data from a continuous month-long operation of GNOME finds no statistically significant signals, thus placing experimental constraints on such dark matter scenarios. 

Abstract Numerous observations suggest that there exist undiscovered beyond‐the‐standard‐model particles and fields. Because of their unknown nature, these exotic particles and fields could interact with standard model particles in many different ways and assume a variety of possible configurations. Here, an overview of the global network of optical magnetometers for exotic physics searches (GNOME), the ongoing experimental program designed to test a wide range of exotic physics scenarios, is presented. The GNOME experiment utilizes a worldwide network of shielded atomic magnetometers (and, more recently, comagnetometers) to search for spatially and temporally correlated signals due to torques on atomic spins from exotic fields of astrophysical origin. The temporal characteristics of a variety of possible signals currently under investigation such as those from topological defect dark matter (axion‐like particle domain walls), axion‐like particle stars, solitons of complex‐valued scalar fields (Q‐balls), stochastic fluctuations of bosonic dark matter fields, a solar axion‐like particle halo, and bursts of ultralight bosonic fields produced by cataclysmic astrophysical events such as binary black hole mergers are surveyed.